Griffith, O. H.2016-05-252016-05-251965-04-15Griffith, O. H. (1965) Electron spin resonance and electronic structure of the RCHOR' ether radicals, J. Chem. Phys. 42, 2651‑2657.https://hdl.handle.net/1794/198818 pagesSingle crystals of inclusion compounds formed between urea and aseries of aliphatic ethers were xirradi ated and studied by electron spin resonance. The stable, x-ray-produced free radicals were all of the general type RCHOR'. The approximate value for the spin density on the carbon atom is 0.70±0.10. The unpaired spm distnbution is discussed in terms of the Hiickel and approximate configuration interaction ^--electron molecular orbital models and the valence bond method. The theoretical spin distributions are found tobe in qualitative agreement with the experimental spin distribution.en-USCreative Commons BY-NC-ND 4.0-USArticle