Cation Exchange Of 1,2,3-Trizolate Metal-Organic Frameworks

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Date

2023-06

Authors

Gombart, Jeffrey Shota

Journal Title

Journal ISSN

Volume Title

Publisher

University of Oregon

Abstract

Cation exchange of various metal salts into cadmium triazolate was explored using methods outlined by Dr. Mircea DincĒŽ, modified for a shorter reaction time. Products were structurally analyzed using PXRD analysis. Cation exchange products maintained the cadmium triazolate structure apart from copper. Several other metal salts would destroy the crystal structure at higher concentrations while copper would do the same at low concentrations. Solvent and temperature studies were done on the copper exchange reaction, determining that bulkier solvents can reduce the reaction energy while increasing reaction temperature had similar effects of increasing metal solvent concentration. Both UV-Vis-NIR analysis as well as SEM-EDX data suggests that our exchange reactions were successful with presence of cobalt and copper in their respective exchange reactions as well as changing metal characteristics in our exchange products.

Description

27 pages

Keywords

material chemistry, metal-organic framework, post synthetic exchange, cation exchange, triazolate

Citation